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  • Author(s):
    Donghoon Han, Garrison M. Crouch, Kaiyu Fu, Lawrence P. Zaino III, Paul W Bohn
    Abstract:

    The ability of zero-mode waveguides (ZMW) to guide light into subwavelength-diameter nanoapertures has been exploited for studying electron transfer dynamics in zeptoliter-volume nanopores under single-molecule occupancy conditions. In this work, we report the spectroelectrochemical detection of individual molecules of the redox-active, fluorogenic molecule flavin mononucleotide (FMN) freely diffusing in solution. Our approach is based on an array of nanopore-confined recessed dual ring elect…

    Date Published:
    2017
    Record Visibility:
    Public