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  • Author(s):
    Prateek Mehta, Patrick Barboun, Yannick Engelmann, David Go, Annemie Bogaerts, William Schneider, Jason Hicks
    Abstract:

    We explore the consequences of nonthermal plasma-activation on product yields in catalytic ammonia synthesis, a reaction that is equilibrium-limited at elevated temperatures. We employ a minimal microkinetic model that incorporates the influence of plasma-activation on N2 dissociation rates to predict NH3 yields into and across the equilibrium-limited regime. NH3 yields are predicted to exceed bulk thermodynamic equilibrium limits on materials that are thermal-rate-limited by N2 dissociation….

    Date Published:
    2020-05
    Record Visibility:
    Public