Search CurateND

Filter by:

Search criteria:

Academic Status: Faculty remove × Creator: Patrick Barboun remove × Creator: Prateek Mehta remove × Creator: Jason Hicks remove × Language: English remove × Type of Work: Article remove ×
Clear all

List of files deposited in CurateND that match your search criteria

  • 1

    Article

    Plasma-Catalytic Ammonia Synthesis beyond the Equilibrium Limit
    Thumbnail
    Author(s):
    Prateek Mehta, Patrick Barboun, Yannick Engelmann, David Go, Annemie Bogaerts, William Schneider, Jason Hicks
    Abstract:

    We explore the consequences of nonthermal plasma-activation on product yields in catalytic ammonia synthesis, a reaction that is equilibrium-limited at elevated temperatures. We employ a minimal microkinetic model that incorporates the influence of plasma-activation on N2 dissociation rates to predict NH3 yields into and across the equilibrium-limited regime. NH3 yields are predicted to exceed bulk thermodynamic equilibrium limits on materials that are thermal-rate-limited by N2 dissociation….

    Date Published:
    2020-05
    Record Visibility:
    Public
  • 2

    Article

    Distinguishing Plasma Contributions to Catalyst Performance in Plasma-Assisted Ammonia Synthesis
    Thumbnail
    Author(s):
    Patrick Barboun, Prateek Mehta, Francisco Herrera, David Go, William Schneider, Jason Hicks
    Abstract:

    Plasma-assisted catalysis is the process of electrically activating gases in the plasma-phase at low temperatures and ambient pressure to drive reactions on catalyst surfaces. Plasma-assisted catalytic processes combine conventional heterogeneous surface reactions, homogeneous plasma phase reactions, and coupling between plasma-generated species and the catalyst surface. Herein, we perform kinetically controlled ammonia synthesis measurements in a dielectric barrier discharge (DBD) plasma-ass…

    Date Published:
    2019-07
    Record Visibility:
    Public
  • 3

    Article

    Distinguishing Plasma Contributions to Catalyst Performance in Plasma-Assisted Ammonia Synthesis
    Thumbnail
    Author(s):
    Patrick Barboun, Prateek Mehta, Francisco Herrera, David Go, William Schneider, Jason Hicks
    Abstract:

    Plasma-assisted catalysis is the process of electrically activating gases in the plasma-phase at low temperatures and ambient pressure to drive reactions on catalyst surfaces. Plasma-assisted catalytic processes combine conventional heterogeneous surface reactions, homogeneous plasma phase reactions, and coupling between plasma-generated species and the catalyst surface. Herein, we perform kinetically controlled ammonia synthesis measurements in a dielectric barrier discharge (DBD) plasma-ass…

    Date Published:
    2019-07
    Record Visibility:
    Public
1 - 3 of 3